Monday, December 04, 2006

Gamma radiation from surface burst fallout and air burst rainout


Above: rainout radiation dangers from air bursts during rainstorms can in certain cases exceed fallout dangers from surface bursts (for a good summary of rainout predictions models, see: A. Schiff, Problems with Predicting Fallout Radiation Hazard in Tactical Battlefield Situations, Lawrence Livermore National Laboratory report UCRL-51440, ADA385024, 1973). A report by W. K. Crandall, et al., An Investigation of Scavenging of Radioactivity from Nuclear Debris Clouds, Lawrence Livermore Laboratory, UCRL-51328 (1973) found that for 15 miles per hour wind, if the whole of the mushroom cloud from a 1 kt air burst was scavenged by rainfall, the peak gamma dose rate at 10 km downwind would be about 25,000 R/hr and would result in an infinite-time accumulated dose of 25,000 R. They found that at 100 km downwind, the peak dose rate from rainout would be 35-100 R/hr and the infinite dose would be 400-1,200 R. For 10 kt, assuming 100% cloud scavenging by rain, they found that the peak dose rate at 10 km downwind would be 70,000 R/hr with an infinite dose of 50,000 R; for 100 km downwind they found 1,500-2,000 R/hr peak dose rate and 10,000-15,000 R dose. For 100 kt, again assuming that 100% of the cloud is scavenged by rain, they found that the peak dose rate at 10 km downwind is 120,000 R/hr with an infinite dose of 80,000 R; at 100 km the peak dose rate is 4,500-5,500 R/hr and the infinite time dose is 30,000-35,000 R. These are far higher dose rates and doses than can occur from land surface bursts, but they are exaggerations for three reasons: (1) less than 100% of the mushroom cloud will be scavenged by rainout because not every fallout particle will be hit by a raindrop, (2) the mushroom cloud will often (especially for higher yields, such as 10-100 kt) rise above the height of the rainclouds, so that only a fraction of the activity can possibly by hit by rain droplets and carried to the ground unless there is a thunderstorm cloud with rain forming at very high altitudes, and (3) the rainout droplets arriving on the surface with fallout particles embedded in the raindrops will generally carry a large fraction of the fallout activity straight down storm sewers, where the gamma radiation is well shielded underground (by two feet of earth or so) from people on the ground. In other words, there is natural decontamination during rainout, unless the drainage is poor and puddles are left.









For previous posts on the topic of fallout from nuclear tests, see here, here, here, here, here, here, etc. The story is that extensive fallout pattern surveyed from the very first nuclear test, Trinity (a low, contaminating, tower burst on 16 July 1945) was covered up in the 1950 edition of Glasstone's official U.S. Department of Defense Effects of Atomic Weapons, which only gave the upwind fallout pattern (excluding the downwind fallout area!).

That same book did however given extensive fallout pattern data for the underwater test Baker, which was deleted from all future editions (1957, 1962/4, and 1977). I want to examine how land surface burst fallout was dealt with by Glasstone and Dolan's official manual from 1957-77.

Fallout prediction in the U.S. Department of Defense's 'The Effects of Nuclear Weapons'

The September 1950 edition, called The Effects of Atomic Weapons, includes a table of Trinity test dose rates from ground zero (it was 8000 R/hr at 1 hour at ground zero) outwards in the upwind (not downwind) direction, without explaining the larger area contaminated downwind than upwind! (The book does have an appendix about fallout plotting using meteorology, and another appendix about calculating dose rates from deposited activity, but doesn’t predict downwind dose rates.) It also has a sequence of detailed fallout and base surge predictions for underwater bursts, based on Baker test data.

The 1957 and 1962/4 editions each have different detailed prediction methods for 20 kt and 1 Mt surface bursts, based on nuclear test data from the Nevada 1951 surface burst Sugar (1.2 kt), with some clever scaling procedures to interpolate with the Eniwetok 1952 surface burst Mike (10.4 Mt) and the Bikini 1954 surface burst Bravo (14.8 Mt). The 1962/4 editions use additional data from 1954 Castle series and 1956 Redwing series tests, for upwind fallout.

The 1957 Effects of Nuclear Weapons fallout prediction for land surface bursts is based on the then-secret and therefore not cited report by D. C. Borg, et al., Radioactive Fallout Hazards from Surface Bursts of Very High Yield Nuclear Weapons, U.S. Armed Forces Special Weapons Project, report AFSWP-507, Secret – Restricted Data, May 1954, which states on page 8:

"Since the Castle Bravo shot [on a coral reef near Namu Island in Bikini Atoll] may be characterized as a hybrid between a land-surface and a water-surface shot, probably most like the former, its ground zero radiation data [which showed relatively low dose rates compared to the Elugelab Island burst Mike shot data] may not be very representative of a true land-surface detonation. For this reason, the Ivy Mike shot has been used as the primary source of data for scaling of radiation effects in the ground zero [upwind] region.

"The downwind fall-out contours constructed for Castle Bravo were based essentially upon survey data taken on the islands involved in the fall-out region."

The 1957 Effects of Nuclear Weapons data for fallout from 20 kt and 1 Mt surface bursts is therefore based on a scaling-based interpolation between 1.2 kt Sugar data and 10.4 Mt Mike data for upwind fallout, and a scaling-based interpolation between 1.2 kt Sugar and 14.8 Mt Bravo data for downwind fallout (no downwind fallout data for Mike was measured).

The scaling system is to scale the linear dimensions of the fallout pattern by the cube-root of the total weapon energy yield, and to scale the dose rate values of contour by both the cube-root of total yield and directly with the fission fraction of the explosion. This derives from the report: Scaling of Contamination Patterns, Surface and Underground Detonations by C. F. Ksanda et al, USNRDL-TR-1, September 15, 1953 (Secret – Restricted Data). The physical basis of this scaling is that the fallout pattern derives from the mushroom cloud, the radioactive parts of which (smaller than the total visible cloud, which is just water vapour at the edges), scale in vertical and horizontal extent by the cube-root of weapon yield. The fallout pattern is then like a "shadow" of the mushroom cloud, so the linear dimensions scale accordingly as the cube-root of yield, while the dose rates for each contour scale according to the depth of fallout which arrives. This fallout depth of deposit is proportional to the cloud’s vertical extent, scaling as the cube root of yield. The confirmation that this scaling system is rigorous is that the total amount of deposited activity within the fallout pattern should be directly proportional to weapon’s fission yield. The scaling confirms this, since the scaled area activity is the scales area, ie the product of two linear scaling factors or (W^{1/3})^2 = W^{2/3}, multiplied by the dose rate scaling factor, which for constant fission fraction is simply W^{1/3}. This product is [W^{2/3}].[W^{1/3}] = W, proving the physical consistency of this whole scaling system.

The 1962/4 editions of The Effects of Nuclear Weapons are different from the 1957 data as regards the prediction of upwind fallout dose rates, which are based on an internal and therefore non cited report by Frank Cluff of the U.S. Weather Bureau, The Upwind Extent of Fallout from a Large Nuclear Detonation, U.S. Department of Commerce, Weather Bureau, Washington, 20 August 1959. This suggests that the fallout dose rate at any point upwind is like rainfall deposition, being dependent on the duration that the mushroom cloud remains overhead (before it is blown downwind and fallout ends), which is about 30 minutes for Bikini and Einwetok bursts in the megaton range (1-15 Mt).

Page 2 of that report states that the data used is: "estimated from Pacific test data [which] gives the up-wind extent for several dose rate contours as a function of total yield based on a 7 knot [8.06 statute miles/hour or 13.0 km/hour] mean tropospheric wind speed and an 80 percent fission yield."

Clearly, therefore, the test data is for low average wind speeds and high average fission yield.
Figure 9.85 on page 455 of the 1962/4 edition of The Effects of Nuclear Weapons shows Cluff’s illustration of the upwind fallout, but it has corrected from Cluff’s case of 7 knots to zero wind by adding 4.03 statute miles to all of the distances of upwind contamination, and has also had the dose rate contours re-scaled to 50% fission instead of Cluff’s case of 80% fission.

If we examine the actual figures, ignoring terrain roughness (which in the Nevada desert reduced the fallout gamma dose rate at 1 m altitude by about 25%) and self-shielding of the instrument by its own battery bulk and by the person holding it (which reduces the observed reading by about another 25%), taking a 1 Mt fission surface burst in a 15 miles/hour wind with 15 degrees of directional shear with altitude from the surface to the mushroom cloud, the predicted dose rate patterns are in fair agreement for a 1 megaton surface burst.

Glasstone 1957 says (empirically) that the 1 hour reference 3000 R/hr contour extends 22 statute miles downwind; the 1962/4 revision states (empirically) that the distance is 23 statute miles, while the 1977 edition based on Dolan's computer simulations using DELFIC and SEER II fallout models gives a distance of 21 miles (ignoring terrain shielding and instrument response). DELFIC in particular is almost entirely non-empirical; the only 'normalization' or 'manual fiddle' introduced empirically into the code was the proportion of the bomb energy which is needed for cloud rise simulations to be accurate (it was found that setting this proportion at 45% gives the observed cloud rise data). The maximum width of this 1 hour 3000 R/hr contour is stated to be 3.1, 6.0, and 2.9 statute miles in the 1957, 1962/4, and 1977 editions, respectively.

In the case of the 1 hour reference 1,000 R/hr contour, the downwind distances are 40, 42, and 40 statute miles, respectively, using the 1957, 1962/4 and 1977 editions, while the corresponding maximum contour widths are 6.8, 10, and 6.9 statute miles, respectively.

At lower dose rates, disagreements are larger. However, the lethal areas where survival demands evacuation or high protection factors by buildings, are most important. Upwind fallout is a particular problem to predict. Most of the empirical data in DASA-1251 for upwind fallout is wrong because the fallout maps of Eniwetok and Bikini have been mis-scaled, as explained in an earlier post. Correcting this error, and you immediately see that the 1952 Mike surface burst produced way higher upwind dose rates than subsequent tests like 1954 Bravo and 1956 Tewa and Zuni, allowing for yield and fission proportion correction factors.

The Mike test produced more severe upwind fallout because of the way the massive steel bomb container modified the fallout distribution process and resultant particle size distribution. This would not occur with stockpiled warheads.

Glasstone 1957 states that a 1 hour reference dose rate of 10 R/hr would occur 9.35 statute miles upwind from a 1 Mt surface burst under a 15 miles/hour wind. This was reduced to 1.7 statute miles in the 1962/4 edition, but was increased to 5.8 statute miles in the 1977 edition. The upwind radius of the 100 R/hr contour at 1 hour was 3.46, -1.3 (ie, 1.3 miles downwind, not upwind!), and 3.5 statute miles according to the 1957, 1962/4, and 1977 editions. (The reason why the 100 R/hr contour is seen to commence downwind of ground zero in the 1962/4 edition stems from the assumption in that edition, on page 454, that the upwind fallout has an average arrival time of 24 minutes, so that under a 15 miles/hour wind it travels 15 * 24/60 = 6 miles downwind while falling. This model is likely wrong because it employs data from the inaccurately scaled fallout patterns in reports like WT-915, and also because it ignores the toroidal downdraft from the periphery of the rising, expanding, vortex fireball, which is entirely different in dynamics from a steady deposit of fallout from the full cloud altitude under ambient winds.)

It must be emphasised that except at ground zero and upwind, fallout dose rates never reach the the 1 hour reference level, which is an extrapolation dose rate based on the total deposit.

For example, the 1000 R/hr of gamma radiation in air 1 hour exposure rate quoted for 40 miles downwind (from 1 megaton fission surface burst on an ideal surface, neglecting instrument response, under a 15 miles per hour wind with 15 degrees shear), has an average arrival time of about (40 miles)/(15 miles/hour) = 2.67 hours, by which time the dose rate will have decayed by a factor of 2.67^1.2 = 3.24.

Hence, the maximum dose rate actually encountered at 40 miles downwind will be no more than 1000/3.24 = 308 R/hr. Terrain roughness on average ground (away from buildings which provide greater shielding) will reduce this to 70% of the ideal smooth surface value, while the shielding by the body of the person taking the measurement would each reduce this again to 75% or so, thus a person holding a radiac (radioactivity detection, identification and computation) survey meter will measure about 308 * 0.7 * 0.75 = 162 R/hr peak exposure rate. Because the instrument response is roughly the same as the bone marrow dose (the bone marrow being shielded by surrounding tissues which absorb around 30% of the gamma exposure outside the body), the instrument reading in a fallout field can be used to assess bone marrow exposure. The infinite time bone marrow dose there, allowing for a 20% reduction in dose due to the much quicker decay rate after 200 days than the t^-1.2 'standard decay law', will be 4 * 2.67 * 162 = 1727 R. This is 11.5 times the 150 R limit you would want to avoid a severe risk of acute sickness leading to mortality. Hence, you would need a protection factor of 11.5 if you were 40 miles downwind from a 1 megaton fission surface burst. Most British brick houses have that protection or higher, as long as you keep away from the outer walls/windows and away from the roof.

A lot of claims were made during the 1980s that fallout protection factors in Britain were exaggerated by the U.K. Home Office method of assessment, which uses an averaged wall thickness to include window effects, instead of treating the windows separately to the brickwork. However, this ignores firstly that the calculations assumed 1 MeV gamma ray energy, when it is known that thermonuclear weapons emit very reduced mean energy gamma rays due to fractionation and the massive contributions from very soft gamma ray emitters like neptunium-239, uranium-240, uranium-237, etc. (due to non-fission neutron captures in the thick uranium-238 'pusher' around the lithium deuteride secondary in the weapons), and secondly, the official civil defence advice was that after the bomb (but before fallout arrives) people should block up window spaces with whatever they can, such as furniture like bookcases.

If people could not do that, the fallout or rainout is visible wherever it is life-threatening, and people have time to evacuate, in the cross-wind direction. The highest dose rate fallout follows low altitude winds that you can get an idea of at ground level from the motion of low level clouds (or the stem of the mushroom, if it is not obscured by local cloud cover). The fallout from the upper parts of the mushroom cannot be assessed so easily unless the mushroom cloud can be seen from the ground, or satellite derived upper wind data is available. However, that fallout generally produces less intense dose rates, albeit over a wider area.

RAINOUT

Rainout is one topic that was substantially expanded in the 1978 and 1981 page changes to the 1972 originally 'secret - restricted data' manual Capabilities of Nuclear Weapons, edited by Philip J. Dolan, Defense Nuclear Agency, DNA-EM-1. Dolan actually did some of the research on rainout himself while at Stanford Research Institute in the 1970s. (He had much earlier done extensive research on the gamma ray spectra of different fission type fallout mixtures, including the effects of fractionation, the decay rate of the fractionated fallout, neutron induced radioactivity due to non-fission capture of neutrons, etc.)

The action of rainout is to speed up the fallout rate. Either small fallout particles get swept out of the air by much larger raindrops (this process is strictly termed 'washout'), or the raincloud and fallout cloud combine, allowing small fallout particles to be captured - as a result of their diffusion in all directions as a result of Brownian motion - by small water droplets, which naturally grow (by collisions, condensation, and turbulent attachment) into large raindrops that can then fall out of the raincloud very rapidly (this two-stage mechanism is correctly called 'rainout').

Most rainfall occurs from rain clouds at altitudes of 2.5-5 km, i.e., from the altitude range which corresponds to the mushroom top altitude for a 2 kt nuclear explosion at low altitude or surface level. Some rain comes from much higher altitudes due to thunderstorms, but this quite rare.

Rainout poses a fallout danger from low yield air bursts which would not be present in dry weather. This can affect troops and cause collateral damage by exposing civilians to radiation.

Where good drainage exists in well designed cities, the rainout danger is less severe than fallout because most of the radioactivity goes straight down the drains, where the radiation it emits is well shielded from people. Eventually most of the radioactivity ends up in sediments, and a small fraction ends is dissolved and enters rivers and the ocean, where it is diluted to insignificance compared to the natural background radiation from potassium-40.

Quantitative calculations of the rainout doses in have been published in two Lawrence Livermore Laboratory reports:

(1) J. B. Knox, T. V. Crawford and W. K. Crandall, Potential Exposures from Low-Yield Free-Air Bursts, Lawrence Livermore Laboratory, report UCRL-51164 (1971). This report calculates that if the raincloud top is at an altitude of 7.8 km, then the percentage of the nuclear mushroom cloud that is subject to rainout is 100% for 1 kt, 80% for 10 kt, and 0% for 100 kt.

It also estimates the infinite time whole body gamma dose in rads due to rainout (assuming no sheltering, and no run off into drains) at various distances downwind. Assuming that 100% of the mushroom cloud is subject to rainout from 1 kt, 10 kt, and 100 kt free air bursts (which would require thunderstorms for the 10 kt and 100 kt examples, because normal rainclouds are not high enough to completely envelop the mushroom cloud for 10 kt or more), a 40 km/hour wind and 15 degrees diffusive shear (as for Dolan, 1972 and Glasstone and Dolan, 1977), the dose at 10 km, 100 km, and 2,000 km downwind from a 1 kt burst would be 25,000 rads (rainout mean deposition time of 15 minutes after burst), 900 rads (rainout mean deposition arrival time of 3 hours), and 0.05 rad.

For 10 kt, the corresponding figures for the same distances are 50,000 rads (rainout mean deposition time of 11 minutes after burst), 11,000 rads (rainout mean deposition time of 1.9 hours), and 2 rads. For 100 kt, the figures are 80,000 rads (rainout mean deposition time of 10 minutes after burst), 30,000 rads (rainout mean deposition time of 1.6 hours), and 30 rads.

These 100% rainout figures only apply to the rainout occurring locally, within a region with the radius of the mushroom cloud. Rainout obviously can, at most, deposit 100% of the airborne radioactivity. If this happens around 10 km downwind, you get a dose there of 30,000 rads, but you then get a dose of 1,000 rads at 100 km, because the atmosphere will then be clear due to the rainout around 10 km downwind. So heavy (100%) rainout ends the fallout pattern within one mushroom cloud radius. Complete rainout always results, therefore, in relatively small, localized 'hotspots' and not a general increase in doses over massive areas within the sort of fallout pattern you get from a surface burst. Although a warm front can result in gentle rain over a wide area, once all radioactivity is deposited the air is cleared, so no further rainout of that radioactivity can occur.

(2) W. K. Crandall, et al., An Investigation of Scavenging of Radioactivity from Nuclear Debris Clouds: Research in Progress, Lawrence Livermore Laboratory, report UCRL-51328 (1973). This shows that the accuracy of the predictions above is greatest near the explosion where the doses are most serious. Accuracy degenerates at large distances where doses are small and effects are less serious. As the yield increases in reality, the percentage of the cloud which is intercepted by rain falls, so above 100 kt there is no serious rainout threat unless a thunderstorm exists at the time of detonation, downwind from the burst.

However, very close to the burst, rainout radioactivity doses from 1-10 kt air bursts can be nearly six times greater - over a small area equal to the mushroom cloud size - than dry fallout at similar distances from a land surface burst. For example, at 10 km downwind from 1 kt air burst complete rainout can produce an infinite time outdoor dose (ignoring drainage and shielding, as in the above estimates) of 25,000 rads, as already discussed. This is nearly six times higher than the equivalent dry fallout dose of 4,400 rads for a 1 kt land surface burst at the same 10 km distance etc. (using Glasstone and Dolan, 1977).

In the vast majority of cases, however, air bursts would be likely to occur in dry weather and deposit no local fallout, causing no imminent threat to life outside of the area of initial effects. The fallout would take many weeks, months and even years to gradually be deposited at very low dose rates (due to decay and dilution due to mixing and diffusion while being blown right around the world every month or so).

Even if there was heavy rainout, most of the rainwater would carry the tiny radioactive particles (mixed with the rain) straight down drains, and 1 metre of earth shields reduces the intensity of 1 MeV gamma rays by a factor of about 300. In fact, the average energy (and thus penetrating power) of fallout is considerably less than 1 MeV, so protection is quite high when fallout does down the drain.

There is an interesting bibliography of fallout computation by Richard Rowland of Kaman Sciences Corporation, California, Fallout Computer Codes: A Bibliographyc Perspective, U.S. Defense Nuclear Agency report DASIAC-SR-93-022, July 1994, database reference AD-A281 905. Six major fallout computer codes, including DELFIC (discussed in a previous post on this blog) are discussed briefly.

Rowland points out that DELFIC uses a lognormal fallout particle size distribution based on ground collected deposits of fallout from nuclear tests Teapot-Ess (1.2 kt, Nevada, 1955; shallow underground test, 20 metres depth of burst) and Small Boy (1.65 kt, Nevada, 1962; near surface burst at 3 metres above the ground). The DELFIC median particle radius is 123 microns (0.123 mm).

Other fallout prediction models use grossly different values, and so make differing predictions of the fallout distribution: WSEG-10 uses a median size of 60 microns, while DNAF-1 uses a median diameter of 229 microns. All the models use a fallout particle density of 2.6 grams per cubic centimetre. Another source of disagreement is the fireball thermal fractionation effect on the early fallout dose rate (the relative condensation rates of different fission product decay chains at different times after burst while fallout is forming). DELFIC rigorously analyses this by calculating contributions from each decay chain and summing them to achieve total dose rate.

As a result, DELFIC results in 67% of the activity being refractory (i.e., condensing before the silicate carrier material which forms the majority of the fallout mass) and this portion of activity is diffused throughout the still molten carrier material of the fallout particles in direct proportion to particle volume. It is soluble and has constant specific activity (activity per unit mass) regardless of particle size. The other 33% is from volatile fission product precursors (with low boiling points so they condense only after the silicate fallout carrier has already solidified), and this can only condense on the outside surface of fallout particles. As a result, the latter is more soluble and scales as the surface area of the particle not as the volume (i.e., specific activity, activity/mass, for volatile nuclides scales inversely with fallout particle radius).

Other fallout models deal badly with this because they ignore the fractionation with particle size and with distance from the detonation. WSEG-10 assumes K = 5180 (R/hr)/(fission kt per square kilometre) at 1 hour after burst, compared to a figure of K = 7770 for SEER3 and 6973 for DNAF-1. All these constant figures are misleading, because fractionation changes this ratio (the composition of the debris depends on particle size) with particle size (and thus with distance) from ground zero. This argument started in the late 1950s. Glasstone's 1957 Effects of Nuclear Weapons stated that the ratio is K = 3,200, the 1962 edition gave a ratio of K = 10,000 and noted that terrain irregularities reduced this by 30%, radiac meter shielding by the operator's body reduced it by another 25%, and only 60% of the fallout occurs locally anyway. Glasstone and Dolan 1977 gave K = 7,500 with the same provisos as the 1962 edition. R. R. Rapp of the RAND Corporation challenged this in his report An Error in the Prediction of Fallout Radiation (RAND report RM-5164-PR, December 1966) when he analysed the data from the 1951 Nevada 1.2 kt surface burst Sugar, which is quite smaller than the fallout prediction for a 1 kt burst in Glasstone and Dolan 1977. For Sugar, K(observed) = 2,330 (R/hr)/(fission kt per square kilometre) at 1 hour after burst, based on the integration of the measured local fallout pattern dose rates over area. Allowing for terrain shielding of deposited radiation by the surface irregularities in a desert (a transmission factor of 0.7) and shielding of the instrument by the person holding it (a transmission factor of 0.75), the for Sugar K(theoretical) = 4,440.

In the 1 kt surface burst Sugar fallout pattern, the 300 R/hr handheld-instrument-measured contour at 1 hour extends only about 1.5 km downwind, and the 100 R/hr contour extends 3.8 km downwind at 1 hour, for a mean vector wind velocity of 46 km/hour. By contrast, Glasstone and Dolan 1977, page 430, predicts a 1 hour dose rate of 3,000 R/hr at 1.5 km downwind for a 24 km/hr wind and 1.8 km downwind for a 46 km/hr wind as in the case of Sugar. Since the Glasstone and Dolan fallout predictions are for a theoretically smooth surface and responsive instrument, their dose rates need to be multiplied by 0.7 for desert terrain shielding and by 0.75 for instrument response when being carried by a person, giving 1,575 R/hr at 1.8 km downwind.

This is still over five times the measured dose rate in the nuclear test. The error is fairly similar for other dose rates. This raises serious concerns that civil defence plans against nuclear terrorism are being based on grossly exaggerated threats, and therefore will probably not be optimal in the event of a disaster.

Interestingly, Rowland also contrasts different assumptions about the decay rate of fractionated fallout, remarking that all the models apart from DELFIC and the EM-1 handbook (1992 edition) use t^{-1.2} for model the dose rate fall with time. DELFIC and EM-1, Rowland states, use a rate equivalent to about t^{-1.26}, this approximation being accurate to within plus or minus 10 percent for times after burst of 15 minutes to 1,000 hours. Obviously this is ignoring the large variations caused by neutron capture in U-238 such as Np-239 and U-237 (which results from the reaction whereby a neutron capture in U-238 is followed by two neutrons being emitted).

There is a complete experimental analysis of the effects of fractionation and neutron induced activity on fallout decay curves in Triffet and LaRivere's weapon test report WT-1317 (1961): highly fractionated (depleted) fallout near ground zero of a land surface burst gamma dose rate decays approximately as t^{-1.2}, but at a few hundred kilometres downwind where there is no significant depletion (and for unfractionated fallout from water surface bursts) the decay rate is approximately t^{-1.26}.

For more information on the dose rate to bomb fraction ratio controversy see the useful report Response to DCPA Questions on Fallout, DCPA Research Report No. 20, 1973 here. For more on the terrain shielding factor in deserts see J. M. Ferguson, Ground Roughness Effects for Fallout-Contaminated Terrain: Comparison of Measurements and Calculations, U.S. Naval Radiological Defense Laboratory, report NRDL-TR-645 (May 1963). Ferguson finds that the terrain roughness in a desert reduces the gamma dose rate by a factor of 0.6-0.7.

To see how such relatively large corrections occur, remember that on a smooth flat infinite surface half the dose rate at 1 m height comes from fallout more than 15 metres away. Then work out the angle that direct radiation from fallout at the mean distance of 15 metres is travelling to you: it is coming to you almost horizontally (only about 12% of the dose rate is from air scattered gamma rays, 88% is direct). Because it is coming almost horizontally from such a large distance, any small irregularities in the ground surface will shield a significant fraction of the radiation. Half the radiation comes from the area of a circle of 15 metres around you, an area of 700 square metres. The bulk of the radiation is not coming vertically upwards from nearby fallout such as that under your shoes, but from a very wide areas horizontally around you.

Another aspect is that if you get in an open trench below the ground surface, you will have a protection factor of about 10 from fallout radiation (i.e., you will be receiving just part of the air scattered exposure coming vertically downwards). The activity in the bottom of the trench is insignificant, just as the activity under your shoes is insignificant as a source of radiation in a fallout field. The significant source is the large surrounding area. Even in a house with no roof or windows and completely contaminated floor area, there will be radiation shielding of the large area contribution surrounding the house. Unlike gas protection, fallout shielding does not require you to keep individual fallout particles outside a house. It is not the ingress of fallout contamination which is the significant issue, but the gamma rays travelling at light speed from a very large area of surrounding ground. Anti-civil defence propaganda claims that houses with broken windows will have no fallout shielding because some fallout particles which are moving horizontally may enter the building, contaminating it. This completely misses the point about radiation shielding.

About 90% of the dose is from radiation coming horizontally from fallout deposited over many hundreds to thousands of square metres surround you. The contribution from fallout deposited under your shoes, or even over the floor of a house, is insignificant in comparison. Misunderstanding this vital point will reduce the efficiency of fallout protection.

A good analysis of this using real fallout experimentally is by C. M. Huddleston, et al., Ground Roughness Effects on the Energy and Angular Distribution of Gamma Radiation from Fallout, U.S. Atomic Energy Commission report CEX-62.81, December 1963. They found that over a cracked but fairly flat dry lake bed the fallout dose rate and angular distribution (using a collimated detector) at 3 ft (0.915 m) height is identical to that at 20 ft height over an ideal smooth surface. Hence the dose rate is 0.67 of that over a smooth surface. For 3 ft above a more rough desert terrain or a plowed field, they found that the dose rate and angular distribution was similar to the ideal theory for 40 ft height, so that the reduction factor was 0.54. Another study using Cs-137 sources for a plowed field gave a reduction factor of 0.45 (C. E. Clifford, Effects of Ground Roughness on the Gamma Dose from Cs-137 Contamination, Defense Research Chemical Laboratories, Report No. 401, Ottawa, March 1963).

***


Review of Jack C. Greene & Daniel J. Strom (Editors, Health Physics Society), Would the Insects Inherit the Earth and Other Subjects of Concern to Those Who Worry About Nuclear War, Pergamon Press, London, 1988, 78pp

This book by Greene and Strom is based on material developed for the Health Physics Society Summer School, 'Health Physics Aspects of Nuclear Attack' held at Southeastern Louisiana University, Hammond, LA, from May 28-June 1, 1984. It is a useful supplement to The Effects of Nuclear Weapons and contains five pages by Philip J. Dolan scientifically discussing the risks of nuclear terrorism (pages 17-21, discussed below).

Jack C. Greene, M.Eng., worked on the Manhattan District at Oak Ridge in World War II, became a member of the U.S. Atomic Energy Commission's Radiation Instrument Branch from 1947-51, and then joined civil defence. From 1962-73 he headed the Post-Attack Research Division of the U.S. Defense Civil Preparedness Agency (DCPA), and in in 1973 he became DCPA's Deputy Assistant Director for Research (see examples of his reports on Fallout Contamination of Food and Water, NATO Civil Defence meeting May 1966 here and Response to DCPA Questions on Fallout, DCPA Research Report No. 20, 1973 here). Dr Daniel J. Strom in 1988 was Assistant Professor of Health Physics, Department of Radiation Health, at the University of Pittsburgh. He received his Ph.D. for dose assessment research in 1984.

Wikipedia comments:

'The strange title of this second book refers to the discovery that cockroaches will withstand 67,500 rem (American variety) or 90,000-105,000 rem (German variety), compared to a human lethal exposure of only about 800 rem [4]. One theory which resulted from these observations on insects was that cockroaches, along with some simple plants and bacteria, would be likely to be the only lifeforms to survive a severe nuclear war. This theory was refuted by experience of the very rapid recovery on isolated islands exposed to close-in heavy fallout and other effects from massive hydrogen bombs at the Bikini Atoll and Eniwetok Atoll, as well as from smaller nuclear weapons in the Nevada Test Site and Australia (Montebello Islands, Maralinga and Emu Field). Full ecological recovery surveys were documented before and after each test series. (For a brief online introduction into some these studies - with specific reference to the ecological effects of the 1.69 megatons Operation Castle Nectar shot, detonated in 1954 on a barge above the crater of the 10.4 megatons Ivy Mike thermonuclear test in Eniwetok Atoll - see [5] and [6].)'

The book has a Foreword in favour of civil defence by Dr Lauriston S. Taylor, Sc.D., of the U.S. National Council on Radiation Protection and Measurements (NCRP). The Biographical Sketches at the end of the book state: 'Dr Taylor has been a leader in the field of radiation protection for more than one-half century, beginning with his appointment as Chairman of the National Committee on Radiation Protection in 1929, and continuing with his position as President of the (renamed) National Council on Radiation and Protection Measurements. He retired in 1977. He is currently [1988] Honorary President of the NCRP. ...'

Dr Taylor's Foreword states: 'I am becoming increasingly convinced that the basic problem centers about the overall ignorance of the general public coupled with an overwhelming deluge of mis-information about some of the simplest facts ... disseminated through our collective media - newspapers, radio, TV, and household magazines.

'Unfortunately, most of the public's information comes through those media which are necessarily highly competitive businesses and must make a profit to survive. By their own admissions, unexciting news is no news, and the often dull and technical discussions associated with Civil Defense make unattractive copy, so they tend to develop and emphasize, often out of context, any unusual, exciting or dramatic tidbits that come to hand ... it is truly amazing how many quickly mount the ladder into full-fledged 'facts'. Even when the right questions are asked, wrong answers are the ones likely to be given, whether through avarice or malice or ignorance. It takes real effort to dig out the real facts.'

On page 40, Dr Howard Maccabee, Ph.D., M.D., responds to the most widespread prejudices:

'I am a radiation oncologist, which means my specialty is cancer. Over the last few years, I have treated over eight hundred cancer patients. In a person's life, or in the family in which it occurs, the experience of cancer, especially if it is a cancer that is not cured, is just as stressful on an individual basis as the event of a nuclear disaster. To my knowledge, of the eight hundred cancer patients that I have treated and that have experienced this stress and grief, there has been only one suicide. The great majority of people, no matter what they have to go through to survive, will fight with every ounce of strength and with every breath to go on living even if they can maintain only a semblance of a quality of life.'

On page 48, Dr Warren K. Sinclair, President of the U.S. National Council on Radiation Protection and Measurements, points out: 'For perspective, according to the 1983 World Almanac, in 1980 there were 1,986,000 deaths in the United States, of which 414,320 were caused by malignant neoplasms (cancers), or about 21 percent.'

A great deal of technical information about alpha radiation hazards in nuclear war is summarised on pages 4-9 by Dr Edward T. Bramlitt, Ph.D., who was the Health Physicist at the Defense Nuclear Agency who was responsible for planning the decontamination of Eniwetok Atoll from 1977-80 after 43 major American nuclear tests there, most of which were surface bursts on barges or islands.

Dr Bramlitt begins by pointing out that although U-235 and U-238 emit alpha particles, they are insignificant compared to plutonium because the shorter half-life of the latter gives it a higher decay rate and hazard. The specific activity (decays per second per kg) of U-235 and U-238 are respectively 30,000 and 190,000 times lower than that of Pu-239, which has a half life of only 24,000 years.

Next, the same basic process which creates Pu-239, ie, neutron capture in U-238 in a reactor and/or in a nuclear explosion, followed by beta decay of U-239 into Np-239 and then into Pu-239, also creates some still heavier isotopes of plutonium such as Pu-240, -241, and -242, due to additional neutron captures. Dr Bramlitt discloses that about 65% of the alpha radioactivity in weapons grade plutonium is from Pu-239, 20% is from Pu-240, and about 15% is initially from Pu-241 (although during storage this rapidly decays, with a 13 years half-life, into Am-241).

Pu-242 is created in non-weapons grade reactor fuel due to its longer irradiation time. The essential point about weapons grade plutonium is precisely the fact that the fuel is removed from the reactor and reprocessed before there has been enough time for much multiple neutron capture, generally after 100 days in the reactor. This maximises the fraction of Pu-239 in the plutonium. Dr Bramlitt points out that neutron capture in U-238 during the nuclear explosion is responsible for the heavy elements in fallout:

'Environmental samples from Rongelap Atoll, which was contaminated primarily by fallout from one thermonuclear weapon test at Bikini Atoll in 1954 [Bravo], were analyzed in 1976 and found to have Am-241 making up about 30 percent of the total alpha activity. ... Pu-241 analyses indicate that Am-241 eventually will comprise about 50 percent of the alpha activity in the Marshall Islands. Following one large nuclear test at Eniwetok Atoll in 1952 [Mike], the amount of Am-241 was reported to be sufficient to eventually account for approximately 80 percent of total alpha activity. ... Pu-238 is a relatively short-lived alpha emitter (88-year half-life) which can be produced by several paths, including (n, 2n) reactions on Pu-239 [ie, the capture of one neutron, followed by the emission of two neutrons]. Pu-238 at Eniwetak Atoll typically accounts for one to ten percent of total alpha activity, although samples associated with some tests showed Pu-238 to be in the range from 30 to 50 percent. ... Bikini and Enewetak samples analyzed in this manner show Pu-240 to account for 50 to 60 percent of combined Pu-239 + Pu-240 activity. ... if 16 nCi are uniformly distributed in the lung and maintained at that level, a dose equivalent rate of 15 rem/yr will result. The maximum permissible concentration in air which leads to this dose rate is 40 picocuries per cubic metre. ... Excess deaths from lung cancers have been observed in studies of animals and people. An excess of neoplasms [abnormal tissue growths, not necessarily malignant] has been found in hamsters at 15 rads of alpha radiation and in a group of miners at cumulative dose to the bronchi of four to nine rads [doses in rads or centigray for alpha radiation are not the same as the dose equivalent in rem or centisieverts because a given dose - energy deposition per unit mass - of alpha radiation is far more ionizing and about more damaging than an equal dose of gamma radiation, so the alpha dose needs to be multiplied by a 'quality factor' of 20 to give the dose equivalent for the purpose of predicting biological effects relative to gamma doses]. A significant excess of lung cancers has been observed in a group of Hiroshima survivors who received 9.8 rads to the lung from gamma and neutron irradiation ... the latent period from radiation exposure to death from lung cancer in people is generally 10 or more years.'

We all use Am-241 in our daily lives, since it is the source used in ionization smoke detectors. The ampha particles emitted by bomb fallout have energy of 5.1-5.5 MeV, resulting in ranges in air of 3.6-4.1 cm. In skin, they have a range of about 35 microns (micrometres), which is less than the average thickness of dead skin on humans, so there is no external hazard from alpha radiation to unbroken skin, and the only risk occurs if contamination enters the body in air, water, food, or through a cut or other damage to skin.

A lung dose rate of 1 millirad per year would result from inhaling air containing 1 femtocurie per cubic metre of alpha emitters like plutonium, or from living in an area where the soil surface is contaminated with 0.2 microcuries per square metre, assuming resuspension of the deposited dust into the air by the wind, and a soil contamination of 13 picocuries per gram in the top centimetre.

Nuclear test data exists for the alpha inhalation risk (page 8). In New York, the Pu-239 concentration in air peaked at 0.45 femtocurie/cubic metre in 1959 (from global fallout after extensive atmospheric nuclear tests by Russia and America in 1958) and peaked at 1.68 in 1963 (from global fallout during even more intense atmospheric nuclear testing by Russia and America in 1962). Because of the cessation of tests at the end of 1962, the air concentration of Pu-239 after 1963 fell rapidly - it was 0.91 in 1964, 0.33 in 1965, and 0.13 in 1966.

The ground deposit of Pu-239 in New York City was also measured: it was 0.2 nanocurie/square metre in 1959 and 0.6 in 1963, rising to 1.5 in 1966. Plutonium soon gets washed out of the atmosphere and enters the deep soil or gets flushed through the drains and enters river or lake deep sediment where it ceases to give rise to biological doses.

Dr Charles J. Bridgman, Professor of Nuclear Engineering at Wright-Patterson Air Force Base, and Dr Arthur T. Hopkins, of the U.S. Air Force, on page 10 disclose that for all nuclear test data for surface bursts, an average of 70% of the radioactivity was distributed throughout the volume of melted fallout particles, and 30% was just on the surfaces of non-melted fallout particles. On page 11 they disclose that the median radius of the lognormal particle size versus activity distribution for low yield surface burst nuclear tests over Nevada desert sand is 50 microns (micrometres) compared to 200 microns for high yield surface bursts on coral rock at Eniwetok and Bikini. The finer the particle size distribution of the natural soil, the smaller the fallout and longer the fallout takes to descend, giving time for much more of the radioactivity to decay in transit during the fallout process before the particles reach the ground. Hence, a nuclear explosion in the air produces no local fallout at all because all the debris condenses into micron-sized particles which take months to years to be deposited, around the world. A surface burst on coarse sand would produce fallout like that from Nevada desert tests, while one on soft rock like coral or limestone would produce larger fallout particles which fallout quickly. A surface burst on hard rock would produce still large fallout particles and faster fallout, some of which would be gravel and rocks, while a surface burst on clay would produce very fine fallout particles more like the global fallout from an air burst. At Hiroshima, the radioactive mushroom had been blown downwind by the time the firestorm with its black rain began 30 minutes to 2 hours later, so there was no significant rainout that contributed to the initial nuclear radiation doses. A firestorm cannot interact with the mushroom cloud because it takes too long to get going.

Dr Conrad V. Chester, of Oak Ridge National Laboratory, on pages 12-13 describes the effects of a nuclear bomb explosion surface burst on a nuclear reactor. A 1-GW nuclear reactor produces 3 kg of plutonium daily. Cooling towers are vulnerable to peak overpressures as low as 1-2 psi, electric power transmission towers and cables can be vulnerable to 3-4 psi if the cables are at right angles to the blast, and auxiliary diesel generators and control rooms may be vulnerable to 25 psi.

However, the pressure vessel containing the nuclear material is very strong and needs an overpressure impulse of about 200 psi-seconds to fracture it, which means a 1 Mt weapon landing at 30-60 metres from the reactor core. If that happens, the core inventory of radioactive material will be added to the nuclear explosion fireball and will add to the fallout. The initial effect is insignificant, since in this case the 1 GW reactor core contents will only increase the 1 Mt bomb gamma dose rate at 1 hour after burst by 1%, but at great times after detonation the reactor debris contribution stands out far more, since it decays more slowly (the short lived nuclides produced in a reactor operating for months are decaying while they are created, but the long lived nuclides accumulate, so the average decay rate of the debris activity surviving from fission in a reactor is slower than the fission product mixture produced in a brief burst in a nuclear bomb).

If a nuclear reactor is hit by 25 psi peak overpressure, the control systems and cooling systems (which rely on auxiliary generators for power if the reactor is shut down) could cause the reactor core to overheat, melt down and may then gradually leak some contamination (this is not the explosive situation which occurred to Chernobyl in 1986). Even when the reactor is shut down, the decaying debris in the core produces a lot of heat which needs to be extracted, unless the design includes an efficient heat sink with natural convection possible.

On pages 17-21, Philip J. Dolan, M.Sc., discusses nuclear terrorism: 'I think it probably is inevitable that a nuclear device will be used by terrorists at some time in the future, either as a serious threat or with an actual explosion ... there is some probability that the acquisition may come about by theft of a weapon rather than by fabrication. ... No doubt, there is enough information available in the open literature to enable a group to build a nuclear warhead ... that would produce somewhere between a few tens of tons and a few kilotons of yield, which would be adequate for their purposes.'

Dolan points out that U-235 is extremely expensive to separate from natural U-238 by gaseous diffusion or centrifuges, while U-233 and Pu-239 must be produced in a nuclear reactor by neutron irradiation of Th-232 and U-238, respectively. The plants required for this would 'probably be beyond the reach of terrorist groups' so theft of nuclear components or of an actual weapon is the major concern:

'Fortunately, the plutonium that is made in power reactors is trapped in the highly radioactive residues of the fuel from which it is made. Plutonium represents only about one-half of one percent of the spent fuel from a light-water power reactor. ... More than a ton of this spent fuel must be processed to obtain enough plutonium for one weapon. ...

'All things considered, it appears that theft of already reprocessed plutonium is the most likely route for the terrorists to obtain the fuel. ... Weapon plutonium typically contains six to eight percent Pu-240 and only trace amounts of Pu-241 and Pu-242. When the reactor is run [for longer periods than when producing weapons grade plutonium] to optimize fuel usage for power production, the heavier isotopes, together with some Pu-238 that is also produced, account for 30 to 35 percent of the plutonium in the spent fuel. Pu-240 and Pu-242 fission spontaneously, producing a continuous neutron background. Pu-241 and [its] daughter products are gamma emitters. ... The neutron background also presents a pre-initiation problem that can significantly complicate the design and production of weapons. ...

'A prime threat would seem to come from some of the smaller countries with relatively undeveloped technological and industrial capabilities. Terrorist activities may appear attractive to the leaders of some of these countries who desire to exert influence beyond their own borders but who lack the military or industrial power to do so. In some cases governments have openly supported terrorist activities, while in other cases strong suspicions of such support exist in spite of denials by the governments concerned. Undoubtedly, some such governments harbor desires for nuclear weapons.'

Dr Robert Ehrlich, Chairman of the Department of Physics, George Mason University, discusses 'nuclear winter' propaganda by 'TAPPS' (R.P. Turco, O.B. Toon, T.P. Ackerman, J.B. Pollack and C. Sagan, Nuclear Winter: Global Consequences of Multiple Nuclear Explosions, in Science, v222, 1983, pp. 1283-92; the acronym TTAPS from the author surnames is deliberately meant to involk the name of the military 'lights out' bugle call, taps) on pages 21-23:

'The postulated drop in temperature following a nuclear war arises due to the blockage of sunlight caused by smoke and dust thrown up into the atmosphere. The smoke arises from fires caused by the nuclear detonations (primarily urban fires), while the dust arises due to the presence of numerous ground burst weapons. ... The rate of rainout of soot and dust depends on the turbulence in the atmosphere. In the TTAPS calculation a kind of temperature inversion results in which there is very little chance for smoke and dust to be removed by rainout. In the actual atmosphere, it seems likely that the patchiness of smoke would cause large thermal gradients and much turbulence leading to a rapid rainout. This effect could lead to a totally negligible temperature decline.

'The large temperature decline in the TTAPS calculation results primarily from smoke rather than dust, since the black soot particles tend to block light more than dust particles. ... In order for 100 megatons to give rise to a large temperature drop, one must assume that 1,000 weapons of 0.1 megaton yield are each delivered against different urban areas causing them all to burn. The TTAPS authors (Turco et al., 1983) recognize this to be a highly artificial scenario ...'

Regarding one 'disastrous' and rather suspect prediction of a 20% reduction in ozone layer thickness by a massive USSR-American nuclear war, the book points out elsewhere that this is merely equal to the natural variations in ozone:

'For purposes of comparison, the effective thickness of the ozone layer during summer is about 20 percent less over Miami than over Seattle.'

Jack C. Greene shows on pages 27-28 how the statistical distribution of fallout over America from a nuclear war would produce a spectrum of dose rate and doses. Assuming that 4,447 megatons of ground surface bursts occurred on the 50 states of the U.S. and had a fission proportion of 50%, that 1 kt of fission products deposited per square mile produces 1,000 R/hr of gamma exposure at the 1 hour reference time over average land with shielding from buildings, people, terrain and ground roughness irregularities, etc., that 80% of the fallout is deposited locally (ie, on the US), and that the land area of the 50 states is 3.6 million square miles, Greene calculates a mean 1-hour dose rate of 500 R/hr. Since the average fallout arrival time for Americans would be 2.25 hours, the mean outside dose over the first four days would be 1,100 R, which is lethal. This is the basic reason why civil defence was needed against fallout in the Cold War.

Using the conversion factor between dose rate and the mean specific activity of Nevada test fallout (5 x 10^14 fissions/gram) on page 20 of Greene's earlier 1973 report, the mean fallout mass deposit over America would be 5 grams per square foot or 54 grams per square metre, which is easily visible. (Similar to pouring 1 kilogram of sugar over a room 4.3 metres wide by 4.3 metres long.) The particles would be felt outside like sand grains bouncing off the hands, arms, and face, and could be heard bouncing off hard surfaces like car roofs, bonnets, and windows.

The statistical variation would not, of course, give everyone 1,100 R. Greene in the 1988 book shows that 10% of the U.S. land area would receive 1-hour dose rates below 110 R/hr and 4-day doses below 170 R, a total of 30% would receive 1-hour dose rates below 220 R/hr and 4-day doses below 330 R, a total of 65% would receive 1-hour dose rates below 520 R/hr and 4-day doses below 830 R, 85% would receive 1-hour dose rates below 990 R/hr and 4-day doses below 1,700 R, and the most contaminated 1% would receive 1-hour dose rates of 1,650-3,300 and 4-day doses of 3,300-10,000 R. (Page 25 of Greene's earlier 1973 report indicates that the maximum dose rates measured at 1 hour after nuclear tests, near ground zero (in the crater and on the lip of the crater) , ranged from 3,000-40,000 R/hr but are not of concern for personnel safety since other lethal effects like blast, heat and initial nuclear radiation would predominate so near ground zero.)

Elsewhere the book shows that the 1 MeV mean gamma ray energy assumed for fallout shielding calculations underestimates the protection factor because that energy is always much higher (more penetrating) than the real gamma ray energy of fallout after nuclear tests, and: 'a group of people sitting back-to-back, and fairly close to each other, would provide a significant amount of "mutual shielding". This would increase the building protection factors by multiplicative factors varying between 1.5 and 3 ... the presence of nearby adjacent structures would provide significant mutual shielding between buildings ... in all cases exposures within structures would be considerably below those predicted for buildings in isolation. Some studies have shown that additional multiplicative protection factors of 2 to 3 are quite reasonable to assume.'

On page 33, Dr Sumner Griffin shows that 75% of all American cattle can be sheltered indoors in barns with food reserves of 85 days on average; the mean protection factor of a barn against gamma radiation is 1.8 if ignoring the mutual shielding of animals by each other and ignoring ground roughness, and the corrected protection factor is about 2.5.

Finally, Dr Kenneth Skrable, Professor of Radiological Sciences at the University of Lowell, explains the mechanism of the neutron bomb on pages 51-2. He explains that the fusion of the hydrogen heavy isotopes deuterium and tritium produces helium-4 plus a neutron plus an energy release of 17.6 MeV, of which 80% (14.1 MeV) is released as the kinetic energy of the neutron and 20% (3.52 MeV) is released as the kinetic energy of the helium atom, leading to the massive neutron radiation and weak fireball of the neutron bomb: 'minimal blast and thermal radiation.'

By contrast, nuclear fission only releases a few percent of the total energy as the kinetic energy of neutrons, so the blast and thermal effects from a predominantly fission weapon exceed those from neutron radiation. Dr Skrable concludes on page 52:

'By replacing fission tactical weapons with neutron weapons, the tactical objective of the weapon will be maintained without the collateral damage and death to civilians outside the area of usefulness. Therefore, the neutron bomb, in fact, may be considered to be a bomb that benefits people, civilian people. ...

'The neutron bomb is a miniature hydrogen bomb. It is to be used as a tactical weapon against invading enemy forces. The civilian population, if ever tactical nuclear weapons had to be employed, should favor the neutron bomb over currently stockpiled fission based tactical weapons.'

The U.S. National Council on Radiation Protection and Measurements (NCRP) Report No. 42, Radiological Factors Affecting Decision-Making in a Nuclear Attack, shows that protracted exposures to radiation - such as fallout - are less dangerous than brief exposure to the same dose. For example, they show that the lethal gamma dose for 50% of humans is 450 R for a week-long exposure, but is about 600 R for a one-month long exposure. Increasing the duration, over which a given amount of radiation is spread, increases the time available for the body's repair mechanisms (both cellular repair and DNA break repair by protein P53) to reduce damage.

Friday, November 24, 2006

Russian ex-spy murdered with alpha radiation from Po-210 in tea in London

Update 22 January 2007: BBC Panorama's documentary 'How To Poison A Spy' reports that radiological surveys of the Po-210 trail throughout the contaminated London hotels and restaurants indicates that the really massive lethal quantity of radioactive Po-210 (several billion becquerels) was administered in the tea Litvinenko drank when he visited the Russians and former KGB men Andrei Lugovoi and Dimitri Kovtun at the London Sushi Bar, Piccadilly Circus, on 16 October 2006. Other contamination elsewhere was much less intense. Litvinenko always drank tea, never alcohol. The tea was ordered for Litvinenko in advance of his arrival, and was then poisoned. When Litvinenko arrived, the poisoned drink was waiting and he drank some - but not all - of it. Therefore he received less than the intended contamination, which is the reason why he took until 24 November 2006 to get a lethal dose from radiation. Because of the 138 days radiological half-life of Po-210, he continued to accumulate substantial radiation doses each day until he died, over a month after being contaminated by the 'spiked' tea. The BBC programme visited Laboratory Number 12, in Moscow which is allegedly the official government poison factory that prepared the Po-210 solution to be administered in Litvinenko's tea. The broadcast programme also reports that recently Russians were officially authorized to pursue enemies overseas.


What will happen if a dirty radioactive terrorist bomb explodes, and the first warning is radiation casualties turning up in hospitals? Well we can guess from recent events surrounding the failure of medics in University College Hospital, London, to diagnose in time Litvinenko's acute radiation poisoning from internal exposure to the heavy metal nuclide polonium-210, the most deadly radioactive material on earth due to its short half-life of about 138 days.

Polonium-210 (Po-210) like plutonium-239 (and everything else if you look far enough, say to supernovae debris) is natural in the sense that it occurs in nature in trace amounts, which is exactly the reason why it was possible for Marie Curie to discover and isolate a tiny amount of it (after years of purification), after starting with a ton of the radioactive uranium ore, pitchblend. Plutonium is also an alpha emitter like Po-210 but plutonium is far less toxic: plutonium was discovered in trace amounts in nature around 1950 by the U.S. Atomic Energy Commission, and has a 24,400 years half life so each atom of that emits only one alpha particle per 35,100 years, which is a comparatively low dose rate.

The average life i.e. the average time taken for a single atom to decay is always 1/(ln 2) = 1.44 times the half-life, which enables you to calculate the specific activity if the half life is known, or to calculate the half-life without waiting for a measurable decrease in the radioactivity, which of course is the situation for long half lives of thousands or billions of years; you simply measure the specific activity in units of:

(decays/second per atom) = Becquerels/atom = Bq/atom = 1/(average life of atom measured in seconds) = (ln 2)/(half-life measured in seconds)

so you can calculate the half-life by measuring the specific activity per radiocative atom in a pure sample of the decaying nuclide (uncontaminated by other isotopes):

half-life (in seconds) = (ln 2)/(specific activity in Bq per atom) = 0.6931/(specific activity in Bq per atom)

Conversely, the specific activity is

specific activity, Bq/atom = 0.6931/(half-life measured in seconds)

Hence, the longer the half-life, the lower the specific radioactivity, and the lower the danger; whereas the shorter the half-life, the more toxic it is.

Summary of radiological incompetence timeline:

21 November: Sun article quotes toxicologist Professor John Henry (who was treating Litvinenko), arguing that Litvinenko was poisoned by radiation. (See below.)

23 November: London Daily Express article (published 24 November) quotes Geoff Bellingan, the director of critical care at University College, London, saying: "Radiation poisoning is ... unlikely." (see below.)

24 November: Litvinenko dies and cause of death is announced as radiation poisoning.

Medical diagnosis by "consensus of experts" is therefore not really any more productive than physics string theory is productive physics due to being done by a "consensus of experts". Neither is science, which is not a matter of consensus in practice (unless you want to risk being herded off a cliff with fellow lemmings), but is a matter of hard facts gathered experimentally.

What they should have done is to have taken samples from the patient and monitored them for alpha, beta, and gamma radiation. A high school physics student learns to measure radiation and identify types of radiation (although isotope identification usually requires more elaborate instruments which measure particle energies, not just types of particle). Incompetence with radiotherapists in Britain has been widely emphasised recently, including the case of the girl with cancer who 17 times received a massive radiation overdose in Glasgow.

You might expect that hospitals in the U.K., particularly in London - where dirty bomb threats of radioactive contamination have been raging for years - would have trained radiological and lab staff with suitable instruments to measure samples for radiation. There are two highly ionising (high LET, linear energy transfer; ie, the radiation gives up its energy quickly in matter to produce high doses): alpha and beta. Gamma rays are more penetrating so they go through matter without being stopped (or imparting energy) so easily.

The BBC report shows typical journalistic incompetence, claiming that Po-210 is natural. Well, Marie Curie who discovered it started from a ton of radioactive pitchblend (good uranium ore) and got 1 gram of radium and only a trace of polonium, after several years work in chemically extracting it from the residue after she had isolated radium. The U.S. Atomic Energy Commission around 1950 announced that it has identified plutonium-239 in pitchblend.

If you look hard enough, everything occurs in nature somewhere (supernovae explosions have neutron densities high enough to create all possible radionuclides), so in that sense, all are "natural", or - rather - the word "natural" becomes a sneer word for journalists to use to cover up natural background radiation variations with location and altitude and instead attack minor variations in that due to human activity.

There is nothing "natural" about the dose of Po-210 which poisoned Litvinenko; intense sources of radiation are easily and quickly measured, and the natural distribution of such things is way too low to ever produce acute radiation syndrome in anyone (long-term risks are another matter).

The London "Sun" newspaper reported on 21 November a claim that Litvinenko had been poisoned by radiation, but got the nuclide wrong: http://www.thesun.co.uk/article/0,,2-2006540128,00.html

"A FORMER Russian spy may have been poisoned with radioactive thallium at a London restaurant, a medical expert said.

"John Henry, a toxicologist treating Alexander Litvinenko, says the former KGB man may need a bone marrow transplant.

"He said: "The thallium is the least of it - the radioactivity seems more important.

"In terms of thallium, I do not think I have see a worse case of this.

"It is too early to say how long it will be before he's out of danger. He is very ill at the moment."

"Prof Henry said it was likely the poison had been swallowed.

"Scotland Yard's counter-terrorism unit is leading the hunt for the culprits.

"A top Moscow politician has admitted Litvinenko may have been poisoned by the KGB.

"Viktor Ilyukhin — deputy chairman of the Russian parliament’s security committee — declared: “I can’t exclude that possibility.”

"He said of the dad of one, whose food is feared to have been spiked at a sushi bar: “That former KGB officer had been irritating the Russian authorities for a long time and possibly knew some state secrets.

“So when our special services got the chance to operate not only inside but outside the country, they decided to get rid of him.”

"Litvinenko, 44, is continuing to fight for life at London’s University College Hospital — guarded by armed police.

"He was in intensive care, with medics putting his chances of survival at 50:50.

"Litvinenko is able to talk and make jokes, but his condition remains serious in intensive care.

"Shocking pictures taken yesterday and released by his family showed the appalling effects of the highly-toxic chemical thallium.

"Litvinenko was pictured pale and weak in his hospital bed — his hair all gone.

"Ravaged ... poisoned ex-KGB man Alexander Litvinenko in London hospital yesterday
Litvinenko’s white cell count — a gauge of his immune system — was nearly zero.

"Prof Henry said damage to his blood cells and bone marrow indicated a radioactive element.


"Exiled Russian tycoon Boris Berezovsky said after visiting Litvinenko for a second time: “He is really in very bad shape.” Countryman Ilyukhin said the former KGB colonel, who fled Moscow for Britain five years ago, may have been targeted for probing a Russian journalist’s murder.

"Anna Politkovskaya — a leading critic of Russian president Vladimir Putin — was gunned down at her Moscow flat.

"Ilyukhin said Litvinenko may have been set “to reveal the truth about Anna Politkovskaya’s assassination”.

"The Kremlin has branded his comments “sheer nonsense”. And one counter-intelligence agent insisted a “hit” by the KGB — now renamed the FSB — would have been more PROFESSIONAL.

"He told a Russian paper: “If it was necessary we would find a different, less fussy and public method to get rid of him.”

Litvinenko was poisoned three weeks ago — but thallium takes around a fortnight to kick in.
The police probe is set to focus on two meetings Litvinenko had on November 1. The first was at a London hotel where he had tea with two Russian men — one a former KGB officer.

"The second meeting was at a sushi bar in Piccadilly with an Italian academic.

"It has emerged that Litvinenko made a secret tape revealing assassinations sanctioned by the Kremlin — in case he was murdered. It was being examined by MI5."


TODAY's "Daily Express" newspaper (24 November 2006, page 17) carries an article written last night (23 November) by John Twomey which states:

"POISON RIDDLE DEEPENS AFTER EX-SPY SUFFERS A HEART ATTACK

"FORMER Soviet spy Alexander Litvinenko was on the brink of death last night as doctors admitted they have no idea what is killing him.

"As Scotland Yard hunted the hitmen, there was speculation that he may have been armed with a new drug unknown to Britain's foremost poison experts.

"Mr Litvinenko's condition deteriorated on Wednesday night after he suffered heart failure at London's University College Hospital. Last night he was on a life support machine. ...

"The ex-KGB colonel, a bitter critic of President Putin, fell ill on November 1 after meeting an ex-KGB major called Vladimir at a London hotel and an Italian academic at a nearby sushi bar.

"Scotland Yard was only called last Friday and there has been confusion ever since over which poison was used.

"Toxicologists brought in to treat the 43-year-old appear to be baffled. Geoff Bellingan, the hospital's director of critical care, said: "We are now convinced that the cause of Mr Litvinenko's condition was not a heavy metal like thallium. Radiation poisoning is also unlikely. {EVER HEARD OF THE SCIENTIFIC METHOD - WHEREBY YOU ACTUALLY CHECK FACTS WITH A SOMETHING CALLED A ZINC SULPHIDE PHOSPHOR SCINTILLATION DETECTOR, OR EVEN AN OBSOLETE SCHOOL-TYPE PHYSICS DEPARTMENT END-WINDOWED GEIGER COUNTER TO FIND OUT WHAT THE FACTS ARE, BEFORE MAKING CONCLUSIONS?} Despite extensive {ISN'T THE WORD YOU MEAN ACTUALLY: INCOMPETENT?} tests, we are still unclear as to the cause of his condition."

Twomey's article proceeds to quote an unnamed security source suggesting that a slow acting poison was administered to give the murders time to escape from the country, and to have "a deterrent effect on dissidents and potential rebels because victims suffer so much pain and their loved ones are forced to look on helplessly as they die an agonising death".

Twomey concludes: "Mr Litvinenko defected to Britain in 2000 and has accused Russia of bombing Moscow and blaming it on Chechen rebels. The Italian he met at the sushi bar, Professor Mario Scaramella, showed him a death list on which both their names appeared."

It is disgusting that the cause, Po-210, was not diagnosed within 24 hours of admission to hospital. They knew he was poisoned, and should have checked his symptoms for all three types of poisoning agent: biological, chemical and radiological. Radiation poisoning is the fastest to check for because any radiation poison sufficient to produce acute effects also is sufficiently intense to be detected in seconds by any suitable radioactivity instrument. The medical profession, who use radiotherapy and x-rays routinely, have no excuse of ignorance in radiation matters, and should have ensure proper checks are made. What would happen if a dirty bomb exploded, or a nuclear explosion at a power plant? How would the medical profession respond? Taking days wondering what each casualty is suffering from, then throwing up their arms in confusion?

Chelating agents have bad side effects, but they offer some possibility of removing heavy metal poisons including radioactive ones, and in a case this bad - if diagnosis had been correctly made before the victim actually died - such measures could have offered a possibility of therapy.

The BBC reports at http://news.bbc.co.uk/1/hi/uk/6180682.stm:

"Radiation found after spy's death

"Mr Litvinenko's condition deteriorated rapidly in hospital.

"Radiation briefing Police probing the death of Russian ex-spy Alexander Litvinenko have found above-normal levels of radiation at three locations in London.

"Mr Litvinenko's death has been linked to the presence of a "major dose" of radioactive polonium-210 in his body.

"Scotland Yard confirmed traces were also found at his home, a sushi bar and a hotel, but the risk to others was said by health experts to be very low.

"The Kremlin has denied UK citizen Mr Litvinenko's claims it was involved.

"The traces were found at the Itsu sushi restaurant in Piccadilly, the Millennium Hotel, Grosvenor Square, and at Mr Litvinenko's home in Muswell Hill, north London, Scotland Yard said.

"Officers are looking at CCTV footage and interviewing witnesses, trying to find out who he met around the time he fell ill on 1 November, said Peter Clarke, head of the Counter Terrorism Command which is leading the investigation.

"Tests are also being carried out at the two London hospitals where Mr Litvinenko had been treated, University College and the Barnet General, the Health Protection Agency said. Professor Pat Troop from the HPA told a news conference Mr Litvinenko would have had to either eaten, inhaled or been given the dose of polonium-210 though a wound.
She said the type of death was an "unprecedented event in the UK".

"RADIATION TYPES

"Alpha particles are stopped by a sheet of paper [this is a generalization based on low energy alphas, some high-energy alpha particles are as penetrating as low-energy beta particles and go through several sheets of paper] and cannot pass through unbroken skin.

"Beta particles are stopped by an aluminium sheet [this is vague and misleading, high energy alphas from Sr-90 decays can go through a couple of millimetres of aluminium or so]

"Gamma rays are stopped by thick lead [this is so vague and imprecise that it is unhelpful]

"Dr Troop said the HPA investigation would also look at the number of people who had come into contact with Mr Litvinenko during his stay in hospital: "We are working with staff to draw up a list, we are working through that," she said. "There will be a minimum of tens of people. He was in hospital for several weeks and a number of staff looked after him."

"As the conference drew to a close, a heckler interrupted saying he was from Ukraine and had also been the victim of poisoning.

"A post-mortem examination on Mr Litvinenko has not been held yet.

"The delay is believed to be over concerns about the health implications for those present at the examination.

"But Roger Cox from the HPA said a large quantity of alpha radiation emitted from polonium-210 had been detected in Mr Litvinenko's urine.

"The Home Office said anybody concerned should contact NHS Direct on 0845 4647, who have been briefed about this issue.

"Meanwhile, the government's civil contingencies committee Cobra has met to discuss the case.
'Sheer nonsense'

"Friends have said Mr Litvinenko was poisoned because of his criticism of Russia.

"In a statement dictated before he died at University College Hospital on Thursday, the 43-year-old accused Russian President Vladimir Putin of involvement in his death.

"Mr Litvinenko had recently been investigating the murder of his friend, Russian journalist Anna Politkovskaya, another critic of the Putin government.

"LITVINENKO TIMELINE

"1 Nov - Alexander Litvinenko meets two Russian men at a London hotel and then meets Italian academic Mario Scaramella at a sushi bar in Piccadilly. Hours later he falls ill and is admitted to Barnet General Hospital
17 Nov - Mr Litvinenko is transferred to UCH
19 Nov - Reports say Mr Litvinenko is poisoned with thallium
21 Nov - A toxicologist says he may have been poisoned with "radioactive thallium"
22 Nov - Mr Litvinenko's condition deteriorates overnight. Thallium and radiation ruled out
23 Nov - The ex-spy dies in intensive care

Litvinenko statement in full
Reaction: Russian's death
Timeline of case in full

"Mr Putin's spokesman Dmitry Peskov reiterated the Kremlin's earlier dismissal of allegations of involvement in the poisoning as "sheer nonsense".

"Mr Putin himself has said Mr Litvinenko's death was a tragedy, but he saw no "definitive proof" it was a "violent death".

"Police have been examining two meetings Mr Litvinenko had on 1 November - one at a London hotel with a former KGB agent and another man, and a rendezvous with Italian security consultant Mario Scaramella, at the sushi restaurant in the West End.

"Mr Litvinenko, who was granted asylum in the UK in 2000 after complaining of persecution in Russia, fell ill later that day.

"In an interview with Friday's Telegraph newspaper, former KGB bodyguard Andrei Lugovoi said he had met Mr Litvinenko at the Millennium Hotel but vigorously denied any involvement in the poisoning.

"Mr Scaramella, who is involved in an Italian parliamentary inquiry into Russian secret service activity, said they met because he wanted to discuss an e-mail he had received."

What is polonium-210?

"What is polonium-210?

"It is a naturally occurring radioactive material that emits highly hazardous alpha (positively charged) particles.

"It was first discovered by Marie Curie at the end of the 19th century.

"There are very small amounts of polonium-210 in the soil and in the atmosphere, and
everyone has a small amount of in their body.

"But at high doses, it damages tissues and organs.

"However the substance, historically called radium F, is very hard for doctors to identify.

"Philip Walker, professor of physics, University of Surrey said: "This seems to have been a substance carefully chosen for its ability to be hard to detect in a person who has ingested it."

"What is the risk to other people from the dose Mr Litvinenko received?

"It cannot pass through the skin, and must be ingested or inhaled into the body to cause damage.

"And because the radiation has a very short range, it only harms nearby tissue, so those who came into contact with him are at very little risk.

"William Gelletly, professor of physics at the University of Surrey, said: "Polonium-210 is very unlikely to have contaminated any staff who treated Mr Litvinenko or anyone who came in contact with him since they would have had to ingest or breathe in the contaminated fluids from his body."

"Professor Dudley Goodhead, Medical Research Council Radiation and Genome Stability Unit, said: "To poison someone much larger amounts are required and this would have to be man-made, perhaps from particle accelerator or a nuclear reactor." "

I've commented at Lubos Motl's blog:

Notice Po-210 has a half-life of 140 days, and is a high-energy alpha emitter. Plutonium-239 for contrast has a half-life of 24,400 years so the specific activity of Po-210 (decays per second or Becquerels, per gram) is way higher. The shorter the half life, the more decays per second!Po-210 was used with beryllium as the neutron source (initiator) in the early 1945 nuclear weapons. Alpha particles hitting beryllium fission it, releasing neutrons. This was responsible for most of the deaths after the Windscale nuclear reactor fire in England in 1957. The pile was producing Po-210 for British nuclear bomb tests in Maralinga, but the government kept that secret, claiming that only iodine-131 had been released. (They didn't want the Americans to know Britain was still using obsolete 1945 nuclear initiator technology!)

UPDATE: for acute radiation syndrome, the maximum duration of effective poisoning is always the smaller than the time between initial symptoms and death. Therefore, he wasn't poisoned over many months, or he would have been in chronic health for many months before dying (there is a report that the police are wasting time on this issue). Litvinenko received a dose over a period of time of less than two weeks. He was probably poisoned during a single meal.

The Po-210 then takes time to become located in tissue and irradiate the tissue with a lethal dose of radiation. This is why the death wasn't instant. It is reported that he had a low blood cell count. After Hiroshima and Nagasaki, and other high-dose accidents, irradiation of bone marrow suppressed the white blood cell count to a minimum about 2-4 weeks after exposure. This is usually when death occurs. There is also a suppression of platelets, and their absence prevents blood clotting properly. The bone marrow irradiation relies - in the case of internal poisoning (rather than x/gamma rays or neutrons) - on Po-210 being deposited in the bone.

So from the symptoms, he received a dose over a short period of time (one meal probably) and he died probably 2-4 weeks after that from acute radiation effects on the blood and lymph systems, and from radiation damage to the cardio-vascular system.

I will just add that Putin is innocent until proved guilty, and we should not seek to blame him just because he is ex-KGB and their methods were murderous. Evidence is required before judgement. Finding traces of impurties in the Po-210 samples recovered from the hotel and the restaurant may enable the source to be identified. Po-210 is licenced and impossible to acquire legally without a licence. It is impossible that the source could be more than a few years old due to the short 138 days half-life. Impurities in the sample will serve as a forensic 'fingerprint' to indicate if the source is controlled by Putin in Russia. Even if Putin is responsible, it might not be possible for Britain to arrest him because the Russians have more military power than we do (more nuclear weapons etc.) so it would be a disaster to even think of doing anything other than going through the UN. I actually think Putin is doing a good job in Russia, he just appears very heavy-handed towards dissenters.

Another thing: the radioactive contamination problem is being confused by the BBC. The dose needed to kill a man from no symptoms to acute radiation syndrome death in a week or two is nothing to do with the dose needed for cancer risks. The BBC reported falsely that anyone else contaminated would have died. This is total nonsense. Long term effects like significantly increased risk of leukemia and lung cancer can occur after very much smaller doses, as proved by studies on exposure to radium, radon, and strontium-90 of human beings (uranium miners, radium watch dial painters in the 1920s, and animals in extensive experiments during the 1950s). In fact, for high-LET alpha particle radiation the bombardment of internal tissue by even a single particle is enough to trigger a cancer risk. (For low-LET radiation like gamma rays there may be a threshold needed to either damage or to simply overwhelm natural radiation repair mechanisms in human cells like protein P53.) Long-term effects from alpha particles require doses millions of times smaller than that administered to Litvinenko. Therefore people who may have inhaled traces could be at enhanced cancer risk. The scientific approach to this is far from the BBC.

BRITAIN'S ITV (INDEPENDENT TV) NEWS GOES THE OTHER WAY TO THE BBC:

http://www.itv.com/news/3a3373b68204c141cf39327179877c14.html:

"Putin attacked after ex-spy's death

"10.28, Sun Nov 26 2006

"Cabinet minister Peter Hain has launched an extraordinary attack on Russia's President Putin following the death of former spy Alexander Litvinenko.

"The outspoken Northern Ireland Secretary, indicated that relations with Moscow had hit a low as he exhorted the Russian president to return to democratic processes.

"Referring to "some murky murders" in recent times, he accused Vladimir Putin of damaging "individual liberty and democracy" in Russia.

"His comments reveal how frosty the relationship between London and Moscow has become following the apparent poisoning of the ex-KGB agent.

"Earlier, the Home Secretary John Reid had confirmed that detectives were now treating the death as "suspicious". Until now police had said they were treating it as an unexplained death.

"Mr Reid said: "As at this stage, they're saying to me that they now regard the death as suspicious. That wasn't the case yesterday, for instance."

"Customers of a restaurant and hotel visited by radiation victim Alexander Litvinenko are facing an anxious wait after giving medical samples for tests.

"A number of them were asked to submit urine for analysis after traces of deadly polonium-210 were discovered at the central London premises. The police are continuing their hunt for the source of the poison.

"The Conservatives have now demanded the Government make a Commons statement over the death.

"Shadow Home Secretary David Davis made the plea and called for cooperation with police inquiries from all concerned, including if necessary the Russian authorities.

"He said: "It is essential that other dissidents living in Britain are reassured about their safety and there are also questions about how Polonium-210 came to be used in Britain."

"Cobra, the Government's emergency planning committee, chaired by Home Office minister Tony McNulty, met on Saturday to discuss the affair.

"Mr Litvinenko died on Thursday night after being exposed to highly toxic radioactive isotope polonium 210 - which if ingested will rapidly lead to organ and tissue damage.

"As a result his hair fell out, his body wasted away and his organs slowly failed.

"In a statement read out after his death, he accused Vladimir Putin of what he believes would be the Kremlin's first political assassination in the West since the Cold War.

"He said: "You may succeed in silencing one man. But a howl of protest from around the world will reverberate, Mr Putin, in your ears for the rest of your life."

"A post-mortem examination of Mr Litvinenko's body has been delayed while a risk assessment is carried out to see if it is safe to perform the procedure and what precautions may be necessary.

"An inquest into his death is expected to be opened in the coming days at St Pancras Coroner's Court in north London.

"Nov 25: Litvinenko death: witness tests to be carried out
"Nov 24: 'Ex-spy killed by radioactive element'"

WHAT IS NUKEGATE? The Introduction to "Nuclear Weapons Effects Theory" (1990 unpublished book), as updated 2025

R. G. Shreffler and W. S. Bennett, Tactical nuclear warfare , Los Alamos report LA-4467-MS, originally classified SECRET, p8 (linked HE...